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In the year 2004 she started dating the actor Brad Pitt during the shooting of Mr. and Mrs. Smith. She adopted a son from Cambodia and named him Maddox in the year 2002. Three years later, she adopted a daughter, Zahara. In the year 2004 Brad Pitt, filed papers to adopted both the children legally.
In 2006, the couple finally had their own daughter and named her Shiloh. In the year 2007 she adopted a 3-year-old boy from a Vietnamese orphanage and named him Pax Thien.